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PUBLICATIONS
1998
García, Lucía; Salvador, María L; Bilbao, Rafael; Arauzo, Jesús
Influence of calcination and reduction conditions on the catalyst performance in the pyrolysis process of biomass Journal Article
In: Energy and Fuels, vol. 12, no. 1, pp. 139–143, 1998, ISSN: 08870624.
@article{Garcia1998,
title = {Influence of calcination and reduction conditions on the catalyst performance in the pyrolysis process of biomass},
author = {Lucía García and María L Salvador and Rafael Bilbao and Jesús Arauzo},
url = {https://pubs.acs.org/sharingguidelines},
doi = {10.1021/ef970097j},
issn = {08870624},
year = {1998},
date = {1998-01-01},
journal = {Energy and Fuels},
volume = {12},
number = {1},
pages = {139--143},
publisher = {American Chemical Society},
abstract = {The influence of several preparation parameters on the performance of a coprecipitated nickel alumina catalyst for use in the pyrolysis of lignocellulosic residues has been studied. The variables considered were calcination temperature (750 and 850 °C), reduction time (1, 2, and 3 h), and hydrogen flow in the reduction step (1740 and 3080 cm3 (STP)/min). The catalyst performance was evaluated on a bench scale plant equipped with a continuous fluidized bed reactor using the Waterloo fast pyrolysis process (WFPP) technology. The biomass used was pine sawdust and the reaction temperature was 650 °C. The results show that when the higher calcination temperature is applied, more severe operating conditions on the reduction process must also be applied, but catalyst sintering can appear when very severe reduction conditions are used.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
García, Lucía; Salvador, María L; Arauzo, Jesús; Bilbao, Rafael
Influence of catalyst weight/biomass flow rate ratio on gas production in the catalytic pyrolysis of pine sawdust at low temperatures Journal Article
In: Industrial and Engineering Chemistry Research, vol. 37, no. 10, pp. 3812–3819, 1998, ISSN: 08885885.
@article{Garcia1998a,
title = {Influence of catalyst weight/biomass flow rate ratio on gas production in the catalytic pyrolysis of pine sawdust at low temperatures},
author = {Lucía García and María L Salvador and Jesús Arauzo and Rafael Bilbao},
url = {https://pubs.acs.org/sharingguidelines},
doi = {10.1021/ie9801960},
issn = {08885885},
year = {1998},
date = {1998-01-01},
journal = {Industrial and Engineering Chemistry Research},
volume = {37},
number = {10},
pages = {3812--3819},
publisher = {American Chemical Society},
abstract = {Pine sawdust catalytic pyrolysis has been studied in a fluidized bed at temperatures of 650 and 700 °C. The experimental work was carried out in a bench-scale plant based on Waterloo Fast Pyrolysis Process (WFPP) technology. The Ni-Al catalyst used was prepared by coprecipitation with a molar ratio 1:2 (Ni-Al) and calcined at 750 °C for 3 h. The catalyst was not reduced prior to the biomass reaction. The influence of the catalyst weight/biomass flow rate ratio (Wl mb) on the product distribution and on the quality of the gas product obtained was analyzed. An increase of the W/mb ratio increases the total gas yield and diminishes the liquid yield. When the W/mb ratio increases, H2 and CO yields increase while CO2, CH4, and C2 yields decrease. For W/mb ratios ≥ 0.4 h, no significant modifications are observed on the initial yields of different gases, and it is confirmed that under these conditions the initial gas composition is similar to that for thermodynamic equilibrium. For W/mb ratios < 0.4 h, a simple first-order kinetic equation has been suggested for H2 and CO formation. textcopyright 1998 American Chemical Society.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}